Monograph:
Arnold Krawietz
Non-Linear Continuum Mechanics of Microemulsions
and Amphiphilic Monolayers
Berlin 2007, 164 pages
ISBN: 978 - 3 - 939430 - 04 - 9
The booklet can be obtained from the author.
The pdf-version of the manuscript can be viewed here
Contents:
Microemulsions are objects of chemical physics
with great theoretical and practical importance. They consist of
curved monomolecular fluid films of amphiphiles
in the nano range, which separate oil from water.
One way of understanding the variety of shapes
and phases is the application of the continuum mechanical theory of
surfaces with bending stiffness. The present
monograph gives a comprehensive treatment within the framework of
full non-linearity. Incorporated are bending
and stretching of the film, the monomeric solubility of the amphiphile
within the bulk fluids, and the influence
of the pressures in the cavities.
While the experimentally confirmed three-phase
coexistence of a microemulsion with an oil and a water excess cannot
be explained on the basis of a linear
bending elasticity approach, the nonlinear setting can predict this phenomenon.
It is demonstrated that a state of prestress
within the amphiphilic film on the microscopic level can give rise to a
symmetry breaking of the mesoscopic bending
energy function and thus allows the existence of an X point in the
macroscopic phase map.